Results of experimental and theoretical studies of a poorly understood phenomenon, an intense emission of ultrafine (nanometer)
aerosols (ENA), are reviewed. In the English-language literature, this phenomenon is commonly referred to as a nucleation
burst. ENA events have been observed on all the continents and throughout the depth of the troposphere, with the number of
corresponding publications growing steadily. Intense and long-lasting ENA events have been studied more or less comprehensively
and in full detail for Northern Europe, with 60 to 70% of observations taken in a forest area in the presence of snow cover
and 10 to 20% in coastal marine areas. Most often, ENA events occur during spring and fall, with 95% of cases in the daytime
and under sunny calm conditions, typical of anticyclones. In ENA events, the concentration of nanoparticles initially grows
rapidly to values of 10
3–10
5 cm
−3. One or two hours later, the so-called nuclei fraction with diameters
D = 3–15 nm is produced. The appearance of the Aitken fraction
D = 20–80 nm and the enlargement of aerosol particles inside the accumulation fraction
D = 80–200 nm may occur during the following 4–6 h. Thus, the cycle of formation and growth of atmospheric aerosol particles
in the size range from a few to hundreds of nanometers is reproduced over 6–8 h. A specific synoptic feature of ENA events
over land is that they occur when the polar air is transported to measuring sites and the temperature difference between day
and light is large. During ENA periods, the formation rate of condensation nuclei with a diameter of 100 nm increases 10-to
100-fold. Important factors of ENA genesis are the “aerosol” and “electric” states of the atmosphere. More intense ENA events
occur at low concentrations of background aerosols in the presence of atmospheric ions of medium mobility with
D = 2–3 nm. The international experiments ACE 1 and 2, BIOFOR 1, 2, and 3, ESUP 2000, QUEST, etc., have not yet provided any
clear answers to the questions about physical and statistical dependences of the time of origin and duration of ENA and new
particle characteristics on the solar and ionized radiation intensity and on the content of minor and biogenic gases. Models
of new particle formation are discussed in the review.
Original Russian Text © V.V. Smirnov, 2006, published in Izvestiya AN. Fizika Atmosfery i Okeana, 2006, Vol. 42, No. 6, pp.
723–748.