Volume 55, Number 2, 214-222, DOI: 10.1007/s11426-011-4405-9

Syntheses of N-sulfonyl-N,N-disubstituted amidines via a three-component free-radical coupling reaction of tertiary amines and arenesulfonyl azides with terminal alkynes

XinWei He, YongJia Shang, JinSong Hu, Kai Ju, Wei Jiang and SuFang Wang

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Abstract

A facile and efficient synthesis of N-sulfonyl-N,N-disubstituted amidines has been achieved via a CuI-catalyzed three-component free-radical coupling reaction of tertiary amines and arenesulfonyl azides with terminal alkynes in the presence of azodiisobutyronitrile (AIBN). The reaction mechanism of this reaction has also been studied.

Keywords  free radical – multicomponent reaction – sulfonyl azide – terminal alkyne

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