Volume 68, Numbers 1-2, 7-11, DOI: 10.1023/A:1019075218358

Polymer growth mode on the heterogeneous Ziegler–Natta catalyst: active sites at the bottom of the growing polymer layer

Seong Han Kim and Gabor A. Somorjai

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Abstract

By alternating the supply of propylene and ethylene monomers, alternating polypropylene and polyethylene films were produced on one model Ziegler–Natta catalyst. This way, we could show that the active polymerization sites remain under the growing polymer films and thus the monomer molecules must transport through the growing polymer to the active sites.

Ziegler–Natta - model catalyst - active site - monomer diffusion - X-ray photoelectron spectroscopy - laser reflection interferometry

This revised version was published online in July 2006 with corrections to the Cover Date.

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