Volume 20, Number 3, 787-796, DOI: 10.1007/s10895-010-0622-4

Synthesis and Fluorescence Properties of Donor-Acceptor-Substituted Novel Dipyrazolo[3,4-b:3′,4′-d]Pyridines (DPP)

Madhukar N. Jachak, Sandeep M. Bagul, Dilip R. Birari, Maruti G. Ghagare, Muddassar A. Kazi, Raghunath B. Toche and Vijayavitthal T. Mathad

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Abstract

A rapid and efficient method for the synthesis of novel dipyrazolo[3,4-b:3′,4′-d]pyridines (DPP) from pyrazolo[3,4-b]pyridine was successfully developed. The DPP derivative was further N-alkylated (6, 8) as well as N-linked with amino acids (13) and their photophysical properties were studied along with N-aryl DPP 4 and observed that the chromophores at C4 position in the aryl ring changed the absorption and emission λmax.

Keywords  Pyrazolo[3,4-b]pyridine - Dipyrazolo[3,4-b:3′,4′-d]pyridines (DPP) - Amino acids linked DPP - Absorption and Emission - Quantum yield - HOMO-LUMO

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