We have performed a comparison of ten models that predict the temporal behavior of laser-induced incandescence (LII) of soot.
In this paper we present a summary of the models and comparisons of calculated temperatures, diameters, signals, and energy-balance
terms. The models were run assuming laser heating at 532 nm at fluences of 0.05 and 0.70 J/cm
2 with a laser temporal profile provided. Calculations were performed for a single primary particle with a diameter of 30 nm
at an ambient temperature of 1800 K and a pressure of 1 bar. Preliminary calculations were performed with a fully constrained
model. The comparison of unconstrained models demonstrates a wide spread in calculated LII signals. Many of the differences
can be attributed to the values of a few important parameters, such as the refractive-index function E(m) and thermal and
mass accommodation coefficients. Constraining these parameters brings most of the models into much better agreement with each
other, particularly for the low-fluence case. Agreement among models is not as good for the high-fluence case, even when selected
parameters are constrained. The reason for greater variability in model results at high fluence appears to be related to solution
approaches to mass and heat loss by sublimation.
PACS 65.80.+n; 78.20.Nv; 42.62.-b; 44.05.+e