Volume 15, Number 3, 185-200, DOI: 10.1007/BF01087021

Ewaldite, a new barium calcium carbonate

Ewaldit, ein neues Barium-Calcium-Karbonat. I. Vorkommen von Ewaldit in syntaktischer Verwachsung mit Mackelveyit
I. Occurrence of ewaldite in syntactic intergrowth with mackelveyite

Gabrielle Donnay, J. D. H. Donnay and M. H. Hey

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Abstract

Mackelveyite type specimens turn out to be polycrystals consisting of two phases in syntactic intergrowth. One phase, for which the name mackelveyite is retained, is lime yellow, but usually shiny black owing to amorphous carbonaceous inclusions. Optically biaxial, nearly uniaxial, it is hexagonal by x-ray diffraction and has the cell dimensions reported byMilton et al. (1965), but its space group isP31m. The other phase, to be called ewaldite, is the major constituent of the polycrystals studied byDesautels (1967) under the name mackelveyite. It is bluish green and crystallizes inP63 mc witha=5.284±7 (1 (2[`11] 0)(2\overline {11} 0) and twin symmetry 6 Ba (Ca0.48 RE0.20 Na0.15 K0.11 Sr0.03 U0.02 \square 0.01 )(CO3 )2 Ba (Ca_{0.48} RE_{0.20} Na_{0.15} K_{0.11} Sr_{0.03} U_{0.02} \square _{0.01} )(CO_3 )_2
. ForZ=2 we obtainDx=3.37 g/cm3, as compared withDm=3.25±5 g/cm3. Electron-probe analysis of polycrystals shows uniform concentration of major elements, thus indicating that we are dealing with two crystalline forms of essentially the same chemical formula. For nearly pure ewaldite we getnE(2[`11] 0)(2\overline {11} 0) und Zwillingssymmetrie 6 Ba (Ca0.48 RE0.20 Na0.15 K0.11 Sr0.03 U0.02 \square 0.01 )(CO3 )2 Ba (Ca_{0.48} RE_{0.20} Na_{0.15} K_{0.11} Sr_{0.03} U_{0.02} \square _{0.01} )(CO_3 )_2
. FürZ=2 erhält manD x=3,37 g·cm–3, das Meßresultat istD m=3,25±±5 g·cm–3. Die Elektronensonden-Untersuchung der Polykristalle zeigt eine gleichmäßige Verteilung der Hauptbestandteile; sie weist folglich darauf hin, daß wir es mit zwei kristallinen Formen mit im wesentlichen gleicher chemischer Formel zu tun haben. Die diffuse Röntgenstreuung zeigt, daß Mackelveyit die schlechter geordnete Struktur ist, so daß Mackelveyit durch eine Ordnungs-Umwandlung in Ewaldit übergeht.

With 4 Figures


Dedicated to ProfessorP. P. Ewald for his 82nd birthday.

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