Volume 47, Number 10, 1864-1867, DOI: 10.1007/BF02494485

The influence of ionic medium on the kinetics of ligand replacement in the Ptdient H2O2+ complex in an aqueous solution

I. V. Mironov

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Abstract

The influence of the ion background (NaClO4, LiClO4, and HClO4) on the kinetics of the reaction PtdientH2O2++X→PtdientX++H2O(X=Cl, Br, I, SCN, and N3) was studied at 25°C by spectrophotometry. Changes in the rate constant with increase in the ionic strength are described by the Debye-Hückel and Gosh-Bjerrum equations. The reaction PtdienCl++H2O→PtdientH2O2++Cl was studied by potentiometry and its rate constant was established to depend weakly on variations of the medium.

Key words  salt effect - effect of medium - platinum(II) complexes - diethylenetriamine

Translated fromIzvestiya Akademii Nauk. Seriya Khimicheskaya, No. 10, pp. 1918–1921, October, 1998.

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